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Enzymatic radiofluorination: Fluorinase accepts methylaza-analogue of SAM as substrate for FDA synthesis.

J Mol Catal B Enzym.. 2013-8;

Maxim E. Sergeev, Federica Morgia, Muhammad R. Javed, Mami Doi, Pei Y. Keng. Crump Institute for Molecular Imaging, Department of Molecular and Medical Pharmacology, University of California Los Angeles, 570 Westwood Plaza, Los Angeles, California, 90095, USA.

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摘要

Methylaza-analogue of S-adenosyl-L-methionine (MeAzaAdoMet) was found to be a substrate for fluorinase. This is the first discovery of a new substrate for fluorinase that can be accessed synthetically in high purity. The activity of fluorinase for the new MeAzaAdoMet and [18F]fluoride ion was 32% in 180 minutes.