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Direct Single-Enzyme Biomineralization of Catalytically Active Ceria and Ceria-Zirconia Nanocrystals.

ACS Nano. 2017; 
Curran Christopher D,Lu Li,Jia Yue,Kiely Christopher J,Berger Bryan W,McIntosh St
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Recombinant Antibody Services (Genscript). The resultant protein sequence is given below: The modified silicatein was expressed from E Get A Quote

摘要

Biomineralization is an intriguing approach to the synthesis of functional inorganic materials for energy applications whereby biological systems are engineered to mineralize inorganic materials and control their structure over multiple length scales under mild reaction conditions. Herein we demonstrate a single-enzyme-mediated biomineralization route to synthesize crystalline, catalytically active, quantum-confined ceria (CeO) and ceria-zirconia (CeZrO) nanocrystals for application as environmental catalysts. In contrast to typical anthropogenic synthesis routes, the crystalline oxide nanoparticles are formed at room temperature from an otherwise inert aqueous solution without the addition of a precipita... More

关键词

CO oxidation,biomineralization,catalysis,ceria,ceria?zirconia,nanoparticle,solid solu